Being the slacker that I am, in SoulSilver, I've done nearly everything up until you battle Red, and yet, I haven't had the opportunity (or memory to prepare) to battle and catch Raikou and Entei. Currently, Raikou's HP are down to the low yellow, yet it still won't keep in an Ultra Ball.
Thus, I have two questions to ask:
i. If I were to try to
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2. Any Pokemon can be caught in any type of PokeBall. It's not impossible, just really difficult.
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2. Nope! Like the others said, the Master Ball will just make it easier than going through the trouble of using the others.
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