Technically the Rani would be a better choice for Hermione because the Doctor and the Master were actually friends with her at some point if I'm remembering correctly.
It's hard to really match the goody-two-shoes-ness of the first Romana though. Plus, she genuinely likes the Doctor, whereas the Rani has absolutely no patience for either of them.
...which is what makes Mark of the Rani so delightful.
The Rani probably wanted to smack the two of them, she probably thought that after all those years of having to be around them, she was out of it when the Academy time was over.
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...which is what makes Mark of the Rani so delightful.
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