You know those moments when you suddenly have a craving for a certain pairing and you go searching for all the good fic that's out there for it? I just had one of those for Simon/River. It's over now, but here are the results of my search. (Note: needless to say, incest. Het. Ohsowrong. Mostly R-ish.)
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The Secret Chord: Twisty pretty wrongness.
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Logos: a wonderfully drawn River. Words don't work for her anymore.
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The Edges of Things: More fic that is oh so wrong. Given summary is "River and Simon have a vivid fantasy life."
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Eros and Agape: Simon/Kaylee from River's pov, which can't help being heartbreaking, another excellent River-voice.
And a vid:
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Universe by SE. To Sarah Slean's "Universe." Lyrical and lovely and oh.